Journal
ADVANCED ENERGY MATERIALS
Volume 7, Issue 20, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201602888
Keywords
energy storage; layered oxides; Li-ion batteries; phase transformations
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Funding
- Northeastern Center for Chemical Energy Storage (NECCES), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012583]
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Although layered lithium oxides have become the cathode of choice for state-of-the-art Li-ion batteries, substantial gaps remain between the practical and theoretical energy densities. With the aim of supporting efforts to close this gap, this work reviews the fundamental operating mechanisms and challenges of Li intercalation in layered oxides, contrasts how these challenges play out differently for different materials (with emphasis on Ni-Co-Al (NCA) and Ni-Mn-Co (NMC) alloys), and summarizes the extensive corpus of modifications and extensions to the layered lithium oxides. Particular emphasis is given to the fundamental mechanisms behind the operation and degradation of layered intercalation electrode materials as well as novel modifications and extensions, including Na-ion and cation-disordered materials.
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