Journal
ADVANCED ENERGY MATERIALS
Volume 7, Issue 23, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201700488
Keywords
anode materials; germanium; lithium-ion batteries; structural design
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Funding
- Australian Research Council (ARC) through an ARC Discovery project [DP1094261]
- China Postdoctoral Science Foundation [2016M592303]
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Germanium-based materials are arousing increasing interest as anodes for lithium-ion batteries, stemming from the intrinsic physical and chemical advantages of germanium. This progress report provides a brief review on the current development of germanium-based materials in lithium storage. The state-of-the-art strategies to achieve enhanced electrochemical properties are highlighted, with their main aim being to resolve the trickiest issue: vast volume changes in germanium during cycling. These strategies include structural modification, modification by surface coating, forming germanium-based alloys, and forming binary or ternary germanium-based composites. The recent work on a novel composite of germanium and tin particles encapsulated in double-concentric carbon hollow spheres is also presented here, with an emphasis on the relationship between structural design and improved performance.
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