Journal
ACS CATALYSIS
Volume 7, Issue 11, Pages 7456-7460Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.7b02777
Keywords
Cobalt; Pincer; Benzimidazole; Alcohol; Dehydrogenative Coupling
Categories
Funding
- European Research Council [ERC AdG 692775]
- Israel Science Foundation
- Planning and Budgeting Committee (PBC)
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Herein, we present the base-metal-catalyzed dehydrogenative coupling of primary alcohols and aromatic diamines to selectively form functionalized 2-substituted benzimidazoles, liberating water and hydrogen gas as the sole byproducts. The reaction is catalyzed by pincer complexes of Earth-abundant cobalt under base-free conditions.
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