Journal
ACS CATALYSIS
Volume 7, Issue 5, Pages 3430-3433Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.7b00756
Keywords
C-H activation; N-H allylation; cobalt; domino reaction; heterocycles
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Funding
- European Research Council under the European Community [307535]
- CSC
- Alexander von Humboldt foundation
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The domino C-H/N-H allylation of aryl imidates was accomplished by a versatile cobalt(III) catalyst. In contrast to a tandem rhodium/palladium catalysis approach, an operationally simple cationic cobalt complex proved effective in the step-economical C-H/N-H functionalization of imidates to directly provide expedient access to decorated vinyl isoquinolines by kinetically relevant C-H activation.
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