Journal
CHEMICAL COMMUNICATIONS
Volume 53, Issue 64, Pages 8964-8967Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc04941b
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Funding
- National Natural Science Foundation of China [21572184, 21472154]
- Natural Science Foundation of Fujian Province of China [2017J06006]
- Fundamental Research Funds for the Central Universities [20720160027]
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The catalytic asymmetric alkylation of the remote, unactivated delta-position of N-alkyl amides was enabled by the combination of visible-light-induced proton-coupled electron transfer, 1,5-hydrogen atomtransfer, and chiral Lewis acid catalysis in up to 82% yield and up to 97% ee.
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