Journal
MATERIALS
Volume 10, Issue 7, Pages -Publisher
MDPI AG
DOI: 10.3390/ma10070837
Keywords
perovskite solar cells; annealing condition; film quality; thermal stability
Categories
Funding
- Natural Science Foundation of China [61604119]
- University Association for Science and Technology in Shaanxi, China [20150103]
- Fundamental Research Funds for the Central Universities [JB151406, JB161101, JB161102]
- China Postdoctoral Science Foundation [2016M602771]
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In this work, efficient mixed organic cation and mixed halide (MA(0.7)FA(0.3)Pb(I0.9Br0.1)(3)) perovskite solar cells are demonstrated by optimizing annealing conditions. AFM, XRD and PL measurements show that there is a better perovskite film quality for the annealing condition at 100 degrees C for 30 min. The corresponding device exhibits an optimized PCE of 16.76% with V-OC of 1.02 V, J(SC) of 21.55 mA/cm(2) and FF of 76.27%. More importantly, the mixed lead halide perovskite MA(0.7)FA(0.3)Pb(I0.9Br0.1)(3) can significantly increase the thermal stability of perovskite film. After being heated at 80 degrees C for 24 h, the PCE of the MA(0.7)FA(0.3)Pb(I0.9Br0.1)(3) device still remains at 70.00% of its initial value, which is much better than the control MAPbI(3) device, where only 46.50% of its initial value could be preserved. We also successfully fabricated high-performance flexible mixed lead halide perovskite solar cells based on PEN substrates.
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