Journal
CHEMICAL COMMUNICATIONS
Volume 53, Issue 65, Pages 9067-9070Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc03468g
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Funding
- A*STAR SERC [R-143-000-648-305]
- National University of Singapore [R-143-000-605-112]
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We present herein a new mode of three-component reactions between isocyanoacetates, amines and 3-formylchromones. Both experimental and DFT studies revealed that this Ag-catalyzed unusual transformation is initiated by a facile aza-Michael addition instead of the conventional imine condensation. This catalytic method enables an efficient synthesis of polysubstituted pyrroles.
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