4.6 Article

Heavy fermion behavior in the quasi-one-dimensional Kondo lattice CeCo2Ga8

Journal

NPJ QUANTUM MATERIALS
Volume 2, Issue -, Pages -

Publisher

NATURE PUBLISHING GROUP
DOI: 10.1038/s41535-017-0040-9

Keywords

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Funding

  1. National Natural Science Foundation of China [11274367, 11522435, 11474330, 11574377]
  2. National Key Research and Development Program of China [2016YFA0300604]
  3. State Key Development Program for Basic Research of China [2015CB921300, 2014CB921500]
  4. Strategic Priority Research Program (B) of the Chinese Academy of Sciences [XDB07020000, XDB07020200, XDB07020100]
  5. Japan Society for the Promotion of Science (JSPS) [15K14133, 16H04501]

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Dimensionality plays an essential role in determining the anomalous non-Fermi liquid properties in heavy fermion systems. So far most heavy fermion compounds are quasi-two-dimensional or three-dimensional. Here we report the synthesis and systematic investigations of the single crystals of the quasi-one-dimensional Kondo lattice CeCo2Ga8. Resistivity measurements at ambient pressure reveal the onset of coherence at T * approximate to 20 K and non-Fermi liquid behavior with linear temperature dependence over a decade in temperature from 2 to 0.1 K. The specific heat increases logarithmically with lowering temperature between 10 and 2 K and reaches 800 mJ/mol K-2 at 1 K, suggesting that CeCo2Ga8 is a heavy fermion compound in the close vicinity of a quantum critical point. Resistivity measurements under pressure further confirm the non-Fermi liquid behavior in a large temperature-pressure range. The magnetic susceptibility is found to follow the typical behavior for a one-dimensional spin chain from 300 K down to T *, and first-principles calculations predict flat Fermi surfaces for the itinerant f-electron bands. These suggest that CeCo2Ga8 is a rare example of the quasi-one-dimensional Kondo lattice, but its non-Fermi liquid behaviors resemble those of the quasi-twodimensional YbRh2Si2 family. The study of the quasi-one-dimensional CeCo2Ga8 family may therefore help us to understand the role of dimensionality on heavy fermion physics and quantum criticality.

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