Journal
ADVANCED FUNCTIONAL MATERIALS
Volume 27, Issue 32, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201606735
Keywords
magnetic refrigeration; magnetocaloric effect; multicaloric effect; phase transition
Categories
Funding
- DFG [SPP 1599, GSC 1070]
- European Community [310748 DRREAM]
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Solid-state magnetic refrigeration is a high-potential, resource-efficient cooling technology. However, many challenges involving materials science and engineering need to be overcome to achieve an industry-ready technology. Caloric materials with a first-order transition-associated with a large volume expansion or contraction-appear to be the most promising because of their large adiabatic temperature and isothermal entropy changes. In this study, using experiment and simulation, it is demonstrated with the most promising magnetocaloric candidate materials, La-Fe-Si, Mn-Fe-P-Si, and Ni-Mn-In-Co, that the characteristics of the first-order transition are fundamentally determined by the evolution of mechanical stresses. This phenomenon is referred to as the stress-coupling mechanism. Furthermore, its applicability goes beyond magnetocaloric materials, since it describes the first-order transitions in multicaloric materials as well.
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