4.7 Article

Isolation of single Pt atoms in a silver cluster: forming highly efficient silver-based cocatalysts for photocatalytic hydrogen evolution

Journal

CHEMICAL COMMUNICATIONS
Volume 53, Issue 68, Pages 9402-9405

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc04061j

Keywords

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Funding

  1. National Natural Science Foundation of China [21573068, 21603073]
  2. Program of Shanghai Subject Chief Scientist [15XD1501300]
  3. Fundamental Research Funds for the Central Universities [222201514303, 222201714001, 222201718002]
  4. China Postdoctoral Science Foundation [2016M591615, 2016M601523, 2017T100276]
  5. National Postdoctoral Program for Innovative Talents [BX201600050]
  6. Shanghai Sailing Program [17YF1402900]
  7. Shanghai Municipal Education Commission
  8. Shanghai Education Development Foundation [16CG31]

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The atomically controlled transition of nanohybrids and their effects on charge-carrier dynamics are highly desirable for fundamental studies in photocatalysis. Herein, for the first time, a method combining atomic monodispersity and single-atom alloy was used to prepare a new form of highly efficient silver-based cocatalysts (Ag-25 & Pt1Ag24) on graphitic carbon nitride, representing a novel photocatalytic system for hydrogen evolution.

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