Journal
CHEMICAL SCIENCE
Volume 8, Issue 2, Pages 1356-1359Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6sc03849b
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Funding
- JSPS
- Global COE Program
- University of Tokyo
- MEXT (Japan)
- Japan Science and Technology Agency (JST)
- Grants-in-Aid for Scientific Research [16H01132] Funding Source: KAKEN
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A new class of chiral bifunctional heterogeneous materials composed of Au/Pd nanoparticles and chiral phosphoric acids as active orthogonal catalysts was prepared by utilizing a facile pseudo-suspension copolymerization method. It was found that this heterogeneous catalyst was capable of facilitating the sequential aerobic oxidation-asymmetric intramolecular aza-Friedel-Crafts reaction between benzyl alcohols and N-aminoethylpyrroles. Moreover, the designed chiral heterogeneous catalyst could be recovered and reused several times without significant loss of activity or enantioselectivity.
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