Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 56, Issue 38, Pages 11326-11353Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201612214
Keywords
CO2 conversion; electrochemistry; heterogeneous catalysis; nanostructured materials; reaction mechanisms
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Funding
- National Key Research and Development Program of China [2016YFB0600901]
- National Science Foundation of China [U1463205, 51302185, 21525626, 21606169]
- China Postdoctoral Science Foundation [0401130003]
- Program of Introducing Talents of Discipline to Universities [B06006]
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The gradually increased concentration of carbon dioxide (CO2) in the atmosphere has been recognized as the primary culprit for the rise of the global mean temperature. In recent years, development of routes for highly efficient conversion of CO2 has received much attention. This Review describes recent progress on the design and synthesis of solid-state catalysts for the electrochemical reduction of CO2. The significance of this catalytic conversion is presented, followed by the general parameters for CO2 electroreduction and a summary of the reaction apparatus. We also discuss various types of solid catalysts based on their CO2 conversion mechanisms. We summarize the crucial factors (particle size, surface structure, composition, etc.) determining the performance for electroreduction.
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