Journal
ADVANCED MATERIALS
Volume 29, Issue 35, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201702268
Keywords
3D porous structures; battery anodes; carbon monoliths; K+ full cells
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Funding
- National Natural Science Foundation of China [51502183, 51402202, 51622208]
- Natural Science Foundation of Jiangsu Province of China [BK20150325, BK20140315]
- Jiangsu Shuangchuang Plan
- Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institutions
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An ultrahigh pyridinic N-content-doped porous carbon monolith is reported, and the content of pyridinic N reaches up to 10.1% in overall material (53.4 +/- 0.9% out of 18.9 +/- 0.4% N content), being higher than most of previously reported N-doping carbonaceous materials, which exhibit greatly improved electrochemical performance for potassium storage, especially in term of the high reversible capacity. Remarkably, the pyridinic N-doped porous carbon monolith (PNCM) electrode exhibits high initial charge capacity of 487 mAh g(-1) at a current density of 20 mA g(-1), which is one of the highest reversible capacities among all carbonaceous anodes for K-ion batteries. Moreover, the K-ion full cell is successfully assembled, demonstrating a high practical energy density of 153.5 Wh kg(-1). These results make PNCM promising for practical application in energy storage devices and encourage more investigations on a similar potassium storage system.
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