4.8 Article

Highly Mobile Two-Dimensional Electron Gases with a Strong Gating Effect at the Amorphous LaAIO3/KTaO3 Interface

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 9, Issue 41, Pages 36456-36461

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.7b12814

Keywords

two-dimensional electron gas; Hall mobility; gating effect; spin relaxation; weak localization; weak antilocalization

Funding

  1. National Basic Research Program of China [2013CB921700, 2016YFA0300701]
  2. National Natural Science Foundation of China [11520101002, 51590880, 11374348, 11134007, 11574376, 11574366]
  3. Key Program of the Chinese Academy of Sciences

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Two-dimensional electron gas (2DEG) at the perovskite oxide interface exhibits a lot of exotic properties, presenting a promising platform for the exploration of emergent phenomena. While most of the previous works focused on SrTiO3-based 2DEG, here we report on the fabrication of high-quality 2DEGs by growing an amorphous LaAlO3 layer on a (001)-orientated KTaO3 substrate, which is a 5d metal oxide with a polar surface, at a high temperature that is usually adopted for crystalline LaAlO3 center dot Metallic 2DEGs with a Hall mobility as high as similar to 2150 cm(2)/(V s) and a sheet carrier density as low as 2 X 10(12) cm(-2) are obtained. For the first time, the gating effect on the transport process is studied, and its influence on spin relaxation and inelastic and elastic scattering is determined. Remarkably, the spin relaxation time can be strongly tuned by a back gate. It is reduced by a factor of similar to 69 while the gate voltage is swept from -25 to +100 V. The mechanism that dominates the spin relaxation is elucidated.

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