Journal
CHEMICAL COMMUNICATIONS
Volume 53, Issue 83, Pages 11403-11406Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc06352k
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Funding
- NSFC [21720102007, 21603278, 21573291]
- STP Project of Guangzhou [201504010031]
- NSF of Guangdong Province [S2013030013474]
- FRF for the Central Universities [17lgpy85]
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Through stepwise post-synthetic spacer insertion and click reactions, six Zr-MOFs with different types and amounts of functional groups have been constructed based on proto-MOF PCN-700. Their gas adsorption capacities and selectivities have been greatly improved and finely tuned, demonstrating the combinatorial effect of pore surface modification and pore space partition.
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