Journal
CHEMICAL COMMUNICATIONS
Volume 53, Issue 90, Pages 12185-12188Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc06375j
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Funding
- Research Fellowship from the Vidyasirimedhi Institute of Science and Technology
- Frontier Research Center
- Thailand Research Fund (TRF) [MRG5980114]
- Junior Research Fellowship Program of the French Embassy in Thailand
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The superior catalytic performance of amine-grafted hierarchical basic FAU-type zeolite nanosheets for the aldol condensation of 5-hydroxymethylfurfural (5-HMF) and acetone (Ac) has been achieved due to the synergistic effect of hierarchical structures, featuring basic active sites together with surface modification. This results in an unprecedented yield of 4-[ 5-(hydroxymethyl) furan-2-yl] but-3-en-2-one (HMB) close to 100%. The catalytic activity can be easily tuned by changing the degree of basicity corresponding to the nature of basic sites and surface modification.
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