Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 9, Issue 47, Pages 41594-41598Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.7b13900
Keywords
CO2-in-water emulsion; metal-organic framework; interface; CO2 reduction; photocatalysis
Funding
- Ministry of Science and Technology of China [2017YFA0403003]
- National Natural Science Foundation of China [21525316, 21673254]
- Chinese Academy of Sciences [QYZDY-SSW-SLH013]
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Here, we propose a CO2/water interfacial route for photocatalytic CO2 conversion by utilizing a metal organic framework (MOF) as both an emulsifier and a catalyst. The CO2 reduction occurring at the CO2/water interface produces formate with remarkably enhanced efficiency as compared with that in conventional solvent. The route is efficient, facile, adjustable, and environmentally benign, which is applicable for the CO2 transformation photocatalyzed by different kinds of MOFs.
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