Journal
CATALYSIS COMMUNICATIONS
Volume 102, Issue -, Pages 89-92Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.catcom.2017.08.032
Keywords
Hemicellulose; HZSM-5; Olefin oligomerization; Fuel
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Funding
- Chinese Academy of Sciences Research Program [XDA07070302]
- Applied Basic Research Programs of Qingdao [15-9-1-72-jch]
- Foundation of State Key Laboratory of High-efficiency Utilization of Coal and Green Chemical Engineering [2016-11]
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The biomass hemicellulose as well as initiating agents (ammonium persulfate and tetramethylethylenediamine) was first used as additive for traditional hydro-thermal synthesis for ZSM-5. The results demonstrate that the addition of biomass hemicellulose and initiating agents make the HZSM-5-Hc-S catalyst have larger BET surface areas, more mesopore structure, and stronger acidity. As a result, the HZSM-5-Hc-S catalyst exhibits high stability for the butene oligomerization with butene conversion of about 90% and diesel selectivity of about 86% during the 72 h time on stream.
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