Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 23, Issue 68, Pages 17157-17165Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201703605
Keywords
ball milling; C-H activation; mechanochemistry; solvent-free
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Funding
- RWTH Aachen University through RWTH Start-up grant - Excellence Initiative of the German federal government [StUpPD_221-16]
- RWTH Aachen University through RWTH Start-up grant - Excellence Initiative of the German state government [StUpPD_221-16]
- RWTH Aachen University through Distinguished Professorship Program - Excellence Initiative of the German federal government
- RWTH Aachen University through Distinguished Professorship Program - Excellence Initiative of the German state government
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The advances made in the mechanosynthesis of inorganic and organometallic complexes and the excellent past developments with metal-catalyzed cross-coupling reactions by high-speed ball milling have sufficienly laid the ground work for the merging of C-H functionalization and mechanochemical techniques. In recent years, the fast development of mechanochemical C-H activation have given us examples of metal-catalyzed olefinations, amidations, halogenations, and oxidative couplings, among others. This concept article will describe some of the events that led to the development of mechanochemical C-H activation, the current state-of-the-art, the present challenges of this merge, and some unique scenarios in which mechanochemistry could complement the traditional solution-based approaches.
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