Journal
APPLIED SURFACE SCIENCE
Volume 425, Issue -, Pages 56-62Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.apsusc.2017.06.248
Keywords
1T-MoS2; h-MoO3; Heterostructures; Photoelectrocatalysis; Supercritical carbon dioxide
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Funding
- Innovation Talents Award of Henan Province [114200510019]
- State Key Laboratory of Chemical Engineering [SKL-ChE-13A04]
- Key program of science and technology from Zhengzhou Bureau of science and technology [121PZDGG213]
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Combining the peculiar properties of different ingredients in one ultimate material is an efficient route to achieve the desired functional materials. Compared to 2H-MoS2, 1T-MoS2 nanosheets display the perfect performance of hydrogen evolution reaction (HER) because of the excellent electronic conductivity. However, how to further realize HER in the visual and near-infrared (NIR) region is a great challenge. Herein, we develop an efficient method to locally pattern h-MoO3 on the ultrathin metallic 1T-MoS2 nanosheets and obtain the novel heterostructures of h-MoO3/1T-MoS2. The enhanced photoelectrochemical performance of the as-prepared heterostructures has been demonstrated. Our study indicates it is originated from the synergistic effect between h-MoO3 and 1T-MoS2, i.e., the strong optical absorption of h-MoO3 in the visible and NIR region, the excellent electronic conductivity of 1T-MoS2 and as well as the efficient separation of the photo-induced carriers from the heterostructures. (C) 2017 Elsevier B.V. All rights reserved.
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