Journal
CHEMICAL COMMUNICATIONS
Volume 53, Issue 97, Pages 13063-13066Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc06958h
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Funding
- National Key R&D Program of China [2016YFA0202902]
- National Natural Science Foundation of China [21572036, 21172045]
- External Cooperation Program of Jiangxi Province [20151BDH80045]
- Department of Chemistry, Fudan University
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A robust magnetic nanoparticle- supported N-heterocyclic carbene-palladacycle has been readily synthesized by directly anchoring the structural defined acenaphthoimidazolylidene palladacycle with a long tail on magnetic nanoparticles (MNPs), and functioned as a solid molecular catalyst and exhibited extremely high catalytic activity towards the challenging Suzuki-Miyaura cross-coupling reactions between less-studied heterocyclic 9-chloroacridine and diverse boronic acids. Remarkably, the catalyst could be used 5 times without obvious loss of activity highlighting the efficiency of our strategy of immobilization of previledged catalysts.
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