Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 56, Issue 50, Pages 15891-15895Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201709087
Keywords
allenes; C-H activation; heterocycles; mechanisms; nickel
Categories
Funding
- European Research Council under the European Commission [307535]
- JASSO
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A unified strategy for nickel(0)-catalyzed C-H allylations, alkenylations, and dienylations has been realized through versatile hydroarylations of allenes with ample scope. Thus, an inexpensive nickel catalyst modified with a N-heterocyclic carbene ligand enabled the direct transformation of C-H bonds of biologically relevant imidazole and purine derivatives with full control of regio- and chemoselectivity.
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