Journal
TETRAHEDRON LETTERS
Volume 58, Issue 51, Pages 4731-4739Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetlet.2017.10.048
Keywords
Desymmetrization; mesa-Dial; Acylation; Oxidation; Horeau-Langenbeck amplification
Categories
Funding
- JSPS KAKENHI [17K05784]
- Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan
- Grants-in-Aid for Scientific Research [17K05784] Funding Source: KAKEN
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The desymmetrization of mesa compounds is one of the most effective strategies for asymmetric synthesis. This digest focuses on recent progress in the desymmetrization of meso-diols and their derivatives. The topics discussed here include methods for the enzymatic acylation of meso-diols and the hydrolysis of meso-diesters, acylation, related reactions of meso-diols with organocatalysts and metal catalysts, the oxidation of meso-diols by enzymes, organocatalysts, and metal catalysts, and the desymmetrization of meso-dicarbamates with metal catalysts. The desymmetrization of meso-diols using tandem reactions is also discussed. (C) 2017 Elsevier Ltd. All rights reserved.
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