Journal
SYNLETT
Volume 28, Issue 20, Pages 2956-2960Publisher
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0036-1589098
Keywords
C-H arylation; palladium catalyst; aryl sulfides
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Funding
- JSPS KAKENHI [JP16H01019, JP16H04109, JP16H06887]
- JST ACT-C Grant, Japan [JPMJCR12ZE]
- Japan Association for Chemical Innovation
- Tokuyama Science Foundation
- Naito Foundation
- Grants-in-Aid for Scientific Research [16H06887, 16H01019] Funding Source: KAKEN
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Benzylic C-H arylation of azaarylmethanes with aryl sulfides has been developed by using a Pd-NHC catalyst and an amide base. Various azaarylmethanes and aryl sulfides were involved in the reaction to afford the corresponding diarylmethanes in good to excellent yields. Moreover, triarylmethane synthesis was accomplished through iterative arylations of 2- or 4-methylpyridine with two different aryl sulfides.
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