Journal
13TH INTERNATIONAL CONFERENCE ON GREENHOUSE GAS CONTROL TECHNOLOGIES, GHGT-13
Volume 114, Issue -, Pages 866-872Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.egypro.2017.03.1229
Keywords
Chilled ammonia; CO2-NH3-H2O system; ternary phase diagrams; process optimization; thermodynamics; kinetics
Funding
- Swiss Commission for Technology and Innovation (CTI) [13973.1]
- Alstom Switzerland Ltd.
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This article gives an overview of our holistic approach for the optimization of the Chilled Ammonia Process by (i) understanding the thermodynamics and kinetics of solid formation in the CO2-NH3-H2O system and finding criticalities with respect to solid formation in the process, and by (ii) exploiting solid formation to reduce the energy penalty of CO2 capture by developing a new process, the Controlled Solid Formation-Chilled Ammonia Process. Recent advances in the construction of phase diagrams as well as in the optimization of the new process are highlighted. (C) 2017 The Authors. Published by Elsevier Ltd.
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