Journal
SENSORS AND ACTUATORS B-CHEMICAL
Volume 245, Issue -, Pages 448-461Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.snb.2017.01.107
Keywords
Single tetrapod; Zinc oxide; Hetero; Ethanol; Nanosensor; Hybrid
Funding
- Alexander von Humboldt Foundation [3-3MOL/1148833 STP]
- University of Petroleum and Energy Studies (UPES), Dehradun, India
- German Research Foundation (DFG) [CRC 1261]
- Government of the Republic of Moldova [45inst-15.817.02.29A]
- EPSRC [EP/K009567/2] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/K009567/2] Funding Source: researchfish
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Fabrication of multifunctional devices based on nano- and microstructures of a single semiconducting oxide is an important step for a better understanding of their maximum sensing properties and the base for the development of bottom-up nanotechnologies. In this work we have fabricated, for the first time devices based on a single or two interconnected ZnO tetrapods (T), doped with Fe and alloyed with Fe2O3 nanoparticles (NPs) and microparticles (MPs) in order to improve their sensing properties towards ultraviolet (UV) sensing and ethanol vapour (EtOH). Compared to pristine ZnO-T improved UV and gas sensing properties of Fe-doped ZnO-T were observed. By Fe2O3-alloying of Fe-doped ZnO-T further improvement in sensing properties was obtained with a reduced influence of the relative humidity (RH) on the sensing response. A gas sensing mechanism was proposed and discussed in detail based on the alloyed Fe2O3 NPs and MPs. The results presented here demonstrate the efficiency of doping and alloying of single ZnO microstructures with other semiconducting oxides to improve their sensing properties, including the decrease in influence of RH on the gas response and the rapidity of the sensors. (C) 2017 Elsevier B.V. All rights reserved.
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