Journal
SCIENCE OF THE TOTAL ENVIRONMENT
Volume 599, Issue -, Pages 400-412Publisher
ELSEVIER
DOI: 10.1016/j.scitotenv.2017.04.195
Keywords
Aerosol components; Direct aerosol radiative forcing; AOD; Short-term time resolution; Seoul megacity
Categories
Funding
- Korea Meteorological Administration Research and Development Program [KMIPA 2015-2050]
- National Research Foundation of Korea (NRF) - Ministry of Science, ICT and future Planning [2015R1A2A1A10053971]
- National Research Foundation of Korea [2015R1A2A1A10053971] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
Ask authors/readers for more resources
The temporal variations (diurnal and seasonal) of the optical properties and direct aerosol radiative forcing (DARF) of different aerosol components (water-soluble, insoluble, black carbon (BC), and sea-salt) were analyzed using the hourly resolution data (PM2.5\) measured at an urban site in Seoul, Korea during 2010, based on a modeling approach. In general, the water-soluble component was predominant over all other components (with a higher concentration) in terms of its impact on the optical properties (except for absorbing BC) and DARF. The annual mean aerosol optical depth (AOD, tau) at 500 nm for the water-soluble component was 0.38 +/- 0.07 (0.06 +/- 0.01 for BC). The forcing at the surface (DARF(SFC)) and top of the atmosphere (DARF(TOA)), and in the atmosphere (DARF(ATM)) for most aerosol components (except for BC) during the daytime were highest in spring and lowest in late fall or early winter. The maximum DARF(SFC) occurred in the morning during most seasons (except for the water-soluble components showing peaks in the afternoon or noon in summer, fall, or winter), while the maximum DARF(TOA) occurred in the morning during spring and/or winter and in the afternoon during summer and/or fall. The estimated DARF(SFC) and DARF(ATM) of the water-soluble component were in the range of -49 to -84 W m(-2) and +10 to +22 W m(-2), respectively. The DARF(SFC) and DARF(ATM) of BC were -26 to -39 W m(-2) and +32 to +51 W m(-2), respectively, showing highest in summer and lowest in spring, with morning peaks regardless of the season. This positive DARF(ATM) of BC in this study area accounted for approximately 64% of the total atmospheric aerosol forcing due to strong radiative absorption, thus increasing atmospheric heating by 2.9 +/- 12 K day(-1) (heating rate efficiency of 39 K day(-1) tau(-1)) and then causing further atmospheric warming. (C) 2017 Elsevier B.V. All rights reserved.
Authors
I am an author on this paper
Click your name to claim this paper and add it to your profile.
Reviews
Recommended
No Data Available