Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 57, Issue 3, Pages 626-646Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201706426
Keywords
energy conversion; energy storage; three-dimensional architectures; transition-metal dichalcogenides
Categories
Funding
- MOE under AcRF [ARC 19/15, MOE2014-T2-2-093, MOE2015-T2-2-057, MOE2016-T2-2-103, MOE2017-T2-1-162]
- AcRF [2016-T1-001-147, 2016-T1-002-051, 2017-T1-001-150]
- NTU under a Start-Up Grant in Singapore [M4081296.070.500000]
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Transition-metal dichalcogenides (TMDs) have attracted considerable attention in recent years because of their unique properties and promising applications in electrochemical energy storage and conversion. However, the limited number of active sites as well as blocked ion and mass transport severely impair their electrochemical performance. The construction of three-dimensional (3D) architectures from TMD nanomaterials has been proven to be an effective strategy to solve the aforementioned problems as a result of their large specific surface areas and short ion and mass transport distances. This Review summarizes the commonly used routes to build 3D TMD architectures and highlights their applications in electrochemical energy storage and conversion, including batteries, supercapacitors, and electrocatalytic hydrogen evolution. The challenges and outlook in this research area are also discussed.
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