Journal
ENVIRONMENTAL SCIENCE & TECHNOLOGY
Volume 49, Issue 8, Pages 5203-5210Publisher
AMER CHEMICAL SOC
DOI: 10.1021/es506095e
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Funding
- National Institute of Environmental Health Sciences [P30-ES000210, P30-ES06096]
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Natural gas extraction, often referred to as fracking, has increased rapidly in the U.S. in recent years. To address potential health impacts, passive air samplers were deployed in a rural community heavily affected by the natural gas boom. Samplers were analyzed for 62 polycyclic aromatic hydrocarbons (PAHs). Results were grouped based on distance' from each sampler to the nearest active well. PAR levels were highest when samplers were closest to active wells. Additionally, PAR levels closest to natural gas activity were an order of magnitude higher than levels previously reported in rural areas. Sourcing ratios indicate that PAHs were predominantly petrogenic, suggesting that elevated PAR levels were influenced by direct releases from the earth. Quantitative human health risk assessment estimated the excess lifetime cancer risks associated with exposure to the measured PAHs. Closest to active wells, the risk estimated for maximum residential exposure was 2.9 in 10 000, which is above the U.S. EPA's acceptable risk level. Overall, risk estimates decreased 30% when comparing results froth samplers closest to active wells to those farthest. This work suggests that natural gas extraction may be contributing significantly to PAHs in air, at levels that are relevant to human health.
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