Journal
APPLIED ORGANOMETALLIC CHEMISTRY
Volume 32, Issue 2, Pages -Publisher
WILEY
DOI: 10.1002/aoc.4097
Keywords
catalytic performance; crystal structure; micro-/nanocrystals; microporous metal-organic framework
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Funding
- National Natural Science Foundation of China [21371058]
- Ministry of Education [A200-C-1101]
- East China University of Science and Technology [YA0157117]
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A new metal-organic framework (MOF), [Zn(ATA)(bpd)] (1Zn) (ATA: 2-aminoterephthalic acid; bpd: 1,4-bis(4-pyridyl)-2,3-diaza-1,3-butadiene), exhibiting a three-dimensional extended porous structure was successfully assembled in a MeOH-H2O solvent system. Under various controlled conditions, 1Zn was obtained in a variety of morphologies such as microspheres, microblocks, microsheets, microplates and microrods. The catalytic performance of the 1Zn microsized MOF was evaluated, and a possible catalytic mechanism was proposed. The flexibility of this MOF assembly strategy for shape control will certainly enhance new potential applications of micro-/nano-MOFs.
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