Journal
PHYSICAL REVIEW LETTERS
Volume 119, Issue 5, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.119.056003
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Funding
- Advanced Research Projects Agency-Energy Integration and Optimization of Novel Ion Conducting Solids (IONICS) program [DE-AR0000774]
- U.S. Department of Energy, Energy Efficiency and Renewable Energy Vehicle Technologies Office [DE-EE0007810]
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We generalize the conditions for stable electrodeposition at isotropic solid-solid interfaces using a kinetic model which incorporates the effects of stresses and surface tension at the interface. We develop a stability diagram that shows two regimes of stability: a previously known pressure-driven mechanism and a new density-driven stability mechanism that is governed by the relative density of metal in the two phases. We show that inorganic solids and solid polymers generally do not lead to stable electrodeposition, and provide design guidelines for achieving stable electrodeposition.
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