4.8 Article

Observation and Control of Laser-Enabled Auger Decay

Journal

PHYSICAL REVIEW LETTERS
Volume 119, Issue 7, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.119.073203

Keywords

-

Funding

  1. X-ray Free Electron Laser Utilization Research Project
  2. Ministry of Education, Culture, Sports, Science, and Technology of Japan (MEXT)
  3. Tohoku University
  4. Dynamic Alliance for Open Innovation Bridging Human, Environment and Materials program
  5. Network Joint Research Center for Materials and Devices (Japan)
  6. MEXT [25286064, 26600111, 16H03881]
  7. MEXT
  8. Japan Science and Technology Agency, JST
  9. CREST [JPMJCR15N1]
  10. Deutsche Forschungsgemeinschaft (DFG) [SFB925/1]
  11. Alexander von Humboldt Foundation
  12. Italian Ministry of Research [RBID08CRXK, PRIN2010ERFKXL_006]
  13. CNR-JSPS
  14. European Union Horizon research and innovation program under Marie Sklodowska-Curie [641789 MEDEA]
  15. Grants-in-Aid for Scientific Research [16H03881] Funding Source: KAKEN

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Single-photon laser-enabled Auger decay (spLEAD) is predicted theoretically [B. Cooper and V. Averbukh, Phys. Rev. Lett. 111, 083004 (2013)] and here we report its first experimental observation in neon. Using coherent, bichromatic free-electron laser pulses, we detect the process and coherently control the angular distribution of the emitted electrons by varying the phase difference between the two laser fields. Since spLEAD is highly sensitive to electron correlation, this is a promising method for probing both correlation and ultrafast hole migration in more complex systems.

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