Journal
PHYSICAL REVIEW A
Volume 98, Issue 4, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.98.043403
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Funding
- Deutsche Forschungsgemeinschaft [MU 2347/6-1, IRTG 2079]
- Aarhus University Research Foundation
- Russian Science Foundation [16-13-10024]
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The desorption of excited rubidium atoms off the surface of helium nanodroplets is studied in detail using femtosecond time-resolved photoion and photoelectron imaging spectroscopy in combination with quantum wave-packet simulations. The good agreement of the measured time-dependent velocity distributions with the simulation when exciting the Rb dopant atoms into the 6p state supports the pseudodiatomic model for the Rb-He droplet interaction, even on the level of quantum wave-packet dynamics. Time-resolved photoelectron spectra reveal the partitioning of excitation energy into the dopant and the droplet degrees of freedom.
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