4.8 Article

17.6% stabilized efficiency in low-temperature processed planar perovskite solar cells

Journal

ENERGY & ENVIRONMENTAL SCIENCE
Volume 8, Issue 8, Pages 2365-2370

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ee01720c

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Funding

  1. European Union Horizon of the Synchornics project [604032]
  2. Fondazione Cariplo [2013-0656]

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We present here a planar perovskite solar cell with a stabilized power conversion efficiency (PCE) of 17.6% at the maximum power point and a PCE of 17% extracted from quasi-static J-V with an open-circuit voltage of 1.11 V. Such excellent figures of merit can be achieved by engineering a solution-processed electron buffer layer that does not require high temperature steps. A compact thin film of perovskite absorber is grown onto a PCBM-based electron extraction layer by implementing a novel two-step procedure which preserves the soluble organic interlayer during the deposition of successive layers. We demonstrate that efficient charge extraction is the key for high steady state efficiency in perovskite solar cells with a highly integrable architecture.

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