Journal
ENERGY & ENVIRONMENTAL SCIENCE
Volume 8, Issue 1, Pages 364-375Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ee02853h
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Funding
- Dutch National Research School Combination Catalysis Controlled by Chemical Design (NRSC-Catalysis)
- National Research Initiative BioSolarCells
- Foundation for Fundamental Research on Matter (FOM)
- RF President's grant [MD-276.2014.3]
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We present a synthetic strategy for the efficient encapsulation of a derivative of a well-defined cobaloxime proton reduction catalyst within a photoresponsive metal-organic framework (NH2-MIL-125(Ti)). The resulting hybrid system Co@MOF is demonstrated to be a robust heterogeneous composite material. Furthermore, Co@MOF is an efficient and fully recyclable noble metal-free catalyst system for light-driven hydrogen evolution from water under visible light illumination.
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