Journal
ENERGY & ENVIRONMENTAL SCIENCE
Volume 8, Issue 3, Pages 855-861Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ee03454f
Keywords
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Funding
- Siemens AG
- European Research Council [ARG 247404]
- European Community [ENERGY.2012.10.2.1, 308997]
- FP7 Future and Emerging Technologies (FET) collaborative project PHOCS [309223]
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Photoelectrochemical reduction of CO2 to CO was driven by a TiO2-protected Cu2O photocathode paired with a rhenium bipyridyl catalyst. Efficient and selective CO evolution was shown to be stable over several hours. The use of protic solution additives to overcome severe semiconductor-to-catalyst charge transfer limitations provided evidence of a modified catalytic pathway.
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