Journal
ORGANIC LETTERS
Volume 19, Issue 7, Pages 1812-1815Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b00583
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Funding
- NSFC [21472186, 21525208]
- Fund for New Technology of Methanol Conversion of Dalian Institute of Chemical Physics (Chinese Academy of Sciences)
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Cobalt(III) and rhodiurn(III) catalysts exhibited complementary scope in C-H amidation of aryl enaminones. The amidation reactions proceeded with broad scope under the assistance of a weakly coordinating and bifunctional enaminone directing group. The electrophilicity of the enaminone group can be further utilized in subsequent hydrolysis-cyclization reactions to afford NH 4-quinolones in telescoping reactions.
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