Journal
ORGANIC LETTERS
Volume 19, Issue 13, Pages 3656-3659Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b01657
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- Agence National de la Recherche (ANR agency) [ANR-15-CE07-0001]
- Agence Nationale de la Recherche (ANR) [ANR-15-CE07-0001] Funding Source: Agence Nationale de la Recherche (ANR)
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A very simple and inexpensive catalytic system based on abundant manganese as transition metal and on an inexpensive phosphine-free bidendate ligand, 2-(aminomethyl)pyridine, has been developed for the reduction of a large variety of carbonyl derivatives with 2-propanol as hydrogen donor. Remarkably, the reaction proceeds at room temperature with low catalyst loading (down to 0.1 mol %) and exhibits a good tolerance toward functional groups. High TON (2000) and TOF (3600 h(-1)) were obtained.
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