Journal
ORGANIC LETTERS
Volume 19, Issue 6, Pages 1478-1481Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b00484
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Funding
- Deutsche Forschungsgemeinschaft (DFG, Emmy Noether Fellowship) [BR 4907/1-11]
- Fonds der Chemischen Industrie (FCI, Ph.D. Fellowship)
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An asymmetric synthesis of the C-11-homoterpenoid (+)-Greek tobacco lactone is developed starting from readily available (R)-linalool. The synthesis is comprised of four operations and features a diastereoablative epoxidation and an oxidative tetrahydropyran formation using vanadium-, palladium-, and selenium-catalyzed cyclizations.
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