Journal
ORGANIC LETTERS
Volume 19, Issue 7, Pages 1824-1827Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b00590
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Funding
- JSPS KAKENHI [JP26708013, JP15H00724]
- Grants-in-Aid for Scientific Research [17H03095, 26708013, 15H00724, 24102007] Funding Source: KAKEN
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The synthesis Of nitrogen cation-doped poly cyclic aromatic hydrocarbons (PAHs) having a variety of counteranions is reported via the trimethylsilyl (TMS)-promoted, intramolecular aromatic nudeophilic substitution (SNAr) reaction of fluoroarenes and pyridine groups. The electrochemical properties and optical properties of the obtained nitrogen cation-doped PAHs were studied in detail, clarifying that they have low-lying LUMO levels and good emission properties derived from. the incorporation of planar N-arylpyridinium moieties.
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