Journal
ORGANIC LETTERS
Volume 19, Issue 19, Pages 5062-5065Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b02262
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Funding
- National Natural Science Foundation of China [21402145, 21432007, 21372179]
- Youth Chen-Guang Science and Technology Project of Wuhan City [2015071704011640]
- Natural Science Foundation of Hubei Province [2014CFB181]
- Fundamental Research Funds for Central Universities [204201710177]
- Important Sci-Tech Innovative Project of Hubei Province [2015ACA058]
- 111 Project of the Ministry of Education of China
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Highly enantioselective pyridine-directed rhodium-catalyzed asymmetric hydrogenation of challenging 1,1-diarylalkenes is achieved by using [Rh(NBD)DuanPhos]BF4 as a precatalyst. Various types of 2-pyridine substituted 1,1-diarylalkenes could be hydrogenated with good to excellent enantioselectivities, which provide an efficient route to the synthesis of pharmaceutically and biologically active compounds containing a 2-pyridyl ethane unit.
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