Journal
ORGANIC LETTERS
Volume 19, Issue 18, Pages 4710-4713Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b01960
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Funding
- National Natural Science Foundation of China [NSFC21502232, NSFC21572272]
- Natural Science Foundation of Jiangsu Province [BK20140655]
- Foundation of State Key Laboratory of Natural Medicines [ZZYQ201605]
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An unprecedented palladium-catalyzed allylic alkylation of pronucleophiles with unactivated skipped enynes has been developed. This method provides a straightforward access to a-wide array of 1,3-dienes without the need to preinstall leaving groups or employ extra oxidants. The reaction exhibited high atom, economy, good functional group tolerance, excellent regioselectivities, and scalability. With D2O as cosolvent, deuterium could be incorporated in high efficiency.
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