Journal
ORGANIC LETTERS
Volume 19, Issue 14, Pages 3915-3918Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b01822
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The synthesis of the presumed structure of aeruginosin KT608A Was accomplished for:the first time. The unusual D-diepi-Choi core was prepared from tyrosine via C-H activation and heterogeneous hydrogenation. Due to differences in the spectral data of synthetic and natural Samples, a revised structure featuring L-diepi-Choi Was proposed, which was synthesized and confirmed to be identical. the basis of these findings; revised Structures: for: six additional aeruginosins (KT608B, KT650, GH553, DA495A, DA511, and K13676) are presented:
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