Journal
ORGANIC LETTERS
Volume 19, Issue 6, Pages 1294-1297Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b00089
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Funding
- National Natural Science Foundation of China [81620108027, 21632008, 21602234, 81220108025]
- Major Project of Chinese National Programs for Fundamental Research and Development [2015CB91 0304]
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Herein, rhodium(III)-catalyzed C-H activation/subsequent [4 + 1] cyclization reactions between benzamides and propargyl alcohols are reported in which propargyl alcohols serve as unusual one carbon units. This title transformation led to a series of isoindolinones bearing a quaternary carbon with moderate to good yields without the requirement for external metal oxidants. Due to the mild and simple reaction conditions, this reaction is compatible with various functional groups.
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