Journal
ORGANIC LETTERS
Volume 19, Issue 15, Pages 4074-4077Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b01851
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Funding
- Ministry of Education (MOE) of Singapore [R-143-000-613-112]
- A*STAR SERC [R-143-000-648-305]
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The first catalytic cascade reaction of activated isocyanides with para-quinone methide-aryl esters is presented. Catalyst-enabled divergent pathways have also been achieved to deliver skeletally diverse products. While Ag catalysis leads to an unprecedented highly diastereoselective synthesis of tricyclic ketals, a simple procedure employing Cu catalysis produces oxazole-containing triarylmethanes in high efficiency through an unexpected C-C bond cleavage.
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