Journal
ORGANIC LETTERS
Volume 19, Issue 7, Pages 1550-1553Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b00361
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Funding
- National Natural Science Foundation of China [21472056, 21602070]
- Fundamental Research Funds for the Central Universities [CCNU15ZX002, CCNU16A05002]
- 111 Project [B17019]
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A highly efficient I-2-proinoted formal [4 + 2] cycloaddition has been developed for the synthesis of 2-acylquinolines from methyl ketones and arylamines using 1,4-dithane-2,5-diol as an ethylene, surrogate. Moreover, the investigation of the mechanism suggested that this reaction occurred via an iodination/Korriblurn oxidation/PoVarov/aromatization sequence. It is noteworthy that the arylamine substrate also played an important role in promotirig the reaction.
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