Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 10, Issue 1, Pages 53-58Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.7b17326
Keywords
graphdiyne; two-dimensional materials; N-doping; interfacial synthesis; diine
Funding
- National Natural Science Foundation of China
- National Young Thousand Talents Program
- Shandong Provincial Natural Science Foundation, China
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We explored the interfacial synthesis of 2D N-graphdiyne films at the gas/liquid and liquid/liquid interfaces. Triazine- or pyrazine-based monomers containing ethynyl group were polymerized through the Glaser coupling reactions at interfaces. Several layered, highly ordered and conjugated 2D N-graphdiyne were obtained. Their structures were characterized by TEM, SEM, AFM, XPS, and Raman spectra. Thin films with minimum thickness of 4 nm could be prepared.
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