Journal
NEW JOURNAL OF CHEMISTRY
Volume 41, Issue 10, Pages 3915-3919Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7nj00105c
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Funding
- National Natural Science Foundation of China [51403100]
- Natural Science Foundation of Jiangsu Province [BK20140949]
- Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institutions
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Three hypercrosslinked conjugated microporous polymers were prepared using Friedel-Crafts reaction based on tetraphenylporphyrin, triphenylamine and tetraphenylmethane with p-dimethoxybenzene as an external crosslinker. The polymers show large surface areas (921 m(2) g(-1)) and CO2 uptake capacity (12.3 wt%). Due to its pi-conjugated structure, the tetraphenylporphyrin based polymer (HCTPP) shows high specific capacitance (179 F g(-1)). Considering their large surface area, high gas uptake capacity, good specific capacitance and facile synthesis method, these materials are promising candidates for carbon capture and energy storage.
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