Journal
COMMUNICATIONS CHEMISTRY
Volume 1, Issue -, Pages -Publisher
NATURE PUBLISHING GROUP
DOI: 10.1038/s42004-018-0098-8
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Funding
- National Science Foundation (NSF) [1462267]
- University of Michigan
- Div Of Civil, Mechanical, & Manufact Inn
- Directorate For Engineering [1462267] Funding Source: National Science Foundation
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Covalent organic frameworks, cross-linked crystalline polymers constructed from rigid organic precursors connected by covalent interactions, have emerged as a promising class of nanoporous materials owing to their highly desirable combination of attributes, including facile chemical tunability, structural diversity, and excellent stability. Despite the distinct advantages offered by three-dimensional covalent organic frameworks, research efforts have predominantly focused on the more synthetically-accessible, two-dimensional variants. Here we present an overview of synthetic approaches to yield three-dimensional covalent organic frameworks, identify synthetic obstacles that have hindered progress in the field and recently-employed methods to address them, and propose alternative techniques to circumvent these synthetic challenges.
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