4.8 Article

Direct Amplitude-Phase Near-Field Observation of Higher-Order Anapole States

Journal

NANO LETTERS
Volume 17, Issue 11, Pages 7152-7159

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.7b04200

Keywords

SNOM; anapole; multipole decomposition; near-field microscopy; all-dielectric nanoparticle

Funding

  1. Deutsche Forschungsgemeinschaft (Germany) [EV 220/2-1]
  2. Russian Science Foundation (Russian Federation) [16-12-10287]
  3. University of Southern Denmark (SDU funding)
  4. Villum Fonden (DarkSILD project)
  5. European Research Council [341054]
  6. Villum Fonden [00011116] Funding Source: researchfish
  7. Russian Science Foundation [16-12-10287] Funding Source: Russian Science Foundation

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Anapole states associated with the resonant suppression of electric-dipole scattering exhibit minimized extinction and maximized storage of electromagnetic energy inside a particle. Using numerical simulations, optical extinction spectroscopy, and amplitude-phase near-field mapping of silicon dielectric disks, we demonstrate high-order anapole states in the near-infrared wavelength range (900-1700 nm). We develop the procedure for unambiguously identifying anapole states by monitoring the normal component of the electric near-field and experimentally detect the first two anapole states as verified by far-field extinction spectroscopy and confirmed with the numerical simulations. We demonstrate that higher-order anapole states possess stronger energy concentration and narrower resonances, a remarkable feature that is advantageous for their applications in metasurfaces and nanophotonics components, such as nonlinear higher-harmonic generators and nanoscale lasers.

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